Skip to main content

Photovoltaics: Photo Generation of Charge Carriers





Up until now we have only described the properties of a system in equilibrium. However, it is important to introduce what happens to a semiconductor when it is illuminated with light.The process of interest is known as photogeneration of charge carriers. Here electron-hole pairs are generated as light is absorbed in a semiconductor. During the course introduction we have already mentioned that mobile electrons and holes are formed in a semiconductor as a result of light absorption. Now, I will explain how this process happens. Here we see a photon incident on a semiconductor. At some point this photon can be absorbed by the material.

Absorption is a process, in which the electromagnetic radiation interacts with atoms of a semiconductor, in particular with the valence electrons.This interaction can lead to a liberation of an electron from a covalent bond. If this happens, a valence electron is excited from an energy state in the valence band to an available energy state in the conduction band. It is important to remember that the excitation of an electron to an energy state in the conduction band leaves an unoccupied energy state in the valence band. This state is then occupied by a hole. Photo-generation results in generation of electron-hole pairs, or in other words, the concentration of mobile electrons and the concentration of holes in the material is increased by the same amount. However, this excitation does not always happen. Photo-generation is limited by energy constraints.

To understand these constraints, we need to look at the bandgap energy of asemiconductor.As you recall from our previous post on band diagrams, there are no available energy statesfor electrons in the band gap.For this reason, only if the photon energy is equal or higher than the energy of the band gap,the photon can be absorbed and an electron-hole pair generated.However, if this requirement is not met, the photon will simply pass through thesemiconductor without being absorbed.You may notice that the photon used in this example is red, whereas the photon that wasabsorbed in the previous examples was blue.This is intentional.Red photons have less energy than blue photons.In this example the red photon’s energy is less than that of the bandgap whereas the bluephoton has energy larger than the bandgap.

But how do we know the energy of a photon?The properties of the electromagnetic radiation emitted from the Sun can be described withthe help of the wave-particle duality concept.As a wave, this radiation propagates at the speed of light and it is characterized by twoparameters.The first is the wavelength, which we denote lambda.It is defined as the distance between two adjacent wave peaks.The second is the frequency, which we denote nu, representing the number of cycles persecond.It is determined as the ratio between the speed of light and wavelength, and it is measuredin Hertz.However, light can be seen also as a flow of particles, which are called photons.The energy of a photon is directly proportional to the product between the frequency andthe Planck’s constant “h”.

Let’s now apply these concepts to determine the minimum energy that is needed to liberatea valence electron in a silicon wafer.The band-gap energy of crystalline silicon is equal to 1.12 eV.This is the minimum amount of energy required for a photon to be absorbed and excite anelectron from an energy state in the valence band to an unoccupied energy state in theconduction band.We can now apply the relationships we just saw to determine the wavelength of theelectromagnetic radiation corresponding to this energy value.Stop the post now and determine the maximum wavelength that can be absorbed bysilicon.Now let’s compare your answer with ours.First of all, we need to the determine the frequency of light, when having an energy of 1.12electron volts.We find that this is 2.7 times 10 to the power of 14 hertz.

Then we can calculate the maximum wavelength of light that can be absorbed by Silicon.It results to be 1110 nanometers.Now let’s see what this means when we want to know which part of the solar spectrum canbe absorbed by crystalline silicon.In this figure you can see the spectral power density of the AM1.5 spectrum in yellow.You also can see the fraction of this spectral power density that can be absorbed by siliconand converted into electricity in a solar cell.This is the brown fraction of the spectrum.The red dashed line represents energy of the band gap of Silicon expressed in wavelength oflight.Only the radiation at lower wavelengths carries enough energy to be absorbed and excite anelectron in crystalline silicon.

Therefore, from the solar spectrum, only the part of the spectrum on the left hand side ofthe dashed line can be absorbed in crystalline silicon.You may also notice that not all of the available energy in this part of the spectrum is usedfor generating electricity by a solar cell.This is due to a process known as thermalization and you will learn more about this in thelight management section of the course.As you can imagine, a semiconductor under illumination will be no longer in an equilibriumstate.Once illuminated, the amount of electrons and holes change with respect to the thermalequilibrium values.As these charges are mobile, we have to understand how these charges move around in thesemiconductor once they are excited.This will be the topic of the next post.

Comments

Popular posts from this blog

Photovoltaics: Band Diagram

In the previous post we discussed silicon, which is the most used material in photovoltaics. In this post, we introduce the band diagram, for which we will use silicon as an example. We will start our discussion of the band diagram with the Bohr model of the silicon atom. In semiconductor materials the outer shell of the atom, which is called the valence shell, is not completely filled. The outer shell of silicon contains 4 out of the possible 8 electrons, which we call valence electrons. As we discussed in the previous post, each silicon atom in a crystalline structure is bonded to four other silicon atoms. The bonds between the silicon atoms are called covalent bonds. These bonds actually consist of two valence electrons that are shared by two silicon atoms. All valence electrons are fixed in the lattice, forming covalent bonds, and are therefore immobile. However, at a temperature above absolute zero, thermal energy is supplied to these miconductor and some of the vale

Solar Cells Losses and Design Part 1

We have discussed some important properties of light and characteristics of the radiation of light by our sun. In this post, we will focus on converting that light to electrical energy. This is done using the photovoltaic effect. Photovoltaics covers the direct conversion of sunlight into electrical energy, by a semiconductor material. The term photovoltaics is derived from the Greek word ‘phos’ which means light, and volt, which refers to electricity, specifically voltage. Volt is a reference to the Italian physicist Alessandro Volta, who invented the battery photovoltaic effect that was discovered in 1839, by the French physicist Emond Becquerel. At the age of 19 Becquerel created the first photovoltaic cell by illuminating platinum electrodes, coated with silver chloride in an acid solution. This device was the first to convert light into electricity. The photovoltaic effect occurs through the generation of a potential difference at the junction of two different material

Black Carbon is Found in the Amazon River after Forest Fires

In addition to the tracks of destruction in the forest, the fires in the Amazon leave traces in the Amazon River and its tributaries. Incomplete burning of tree wood results in the production of a type of carbon - known as black carbon - that reaches Amazonian waters in the forms of charcoal and soot and is transported to the Atlantic Ocean as dissolved organic carbon. An international group of researchers quantified and characterized, for the first time, the black carbon that flows through the Amazon River. The results of the study, published in Nature Communications magazine, showed that most of the material transferred to the ocean is "young," suggesting that it was produced by recent forest fires. "We found through radiometric dating analysis [a method that uses the radioisotope of natural carbon-14 occurrence to determine the age of carbonaceous materials up to about 60,000 years] and molecular composition that the largest proportion of the black carbon we found